In 2009, she donated the short story Last (previously published in the Manchester Review Online) to Oxfam's 'Ox-Tales' project, four collections of UK stories written by 38 authors. Her story was published in the 'Fire' collection.
Ali Smith partnered with the Scottish band Trashcan Sinatras and wrote the lyrics to a song called "Half An Apple", a love song about keeping half an apple spare for a loved one who is gone. The song was released on 5 March 2007, on the album Ballads of the Book.
In 2011 she wrote a short memoir for The Observer in their "Once upon a life" series 'Looking back on her life, writer Ali Smith returns to the moment of conception to weave a poignant and funny memoir of an irreverent father, a weakness for Greek musicals and a fateful border crossing' online text here.
In October 2012, she read a sermon at Manchester Cathedral to guests and students, followed by a book signing
In 2013, Smith published Artful, a book based on her lectures on European comparative literature delivered the previous year at Saint Anne's College, Oxford. Much more than a work of literary criticism, it is a book about what art can do. Artful was well-received, with one reviewer commenting that, "...her new book, in which she tugs at God’s sleeve, ruminates on clowns, shoplifts used books, dabbles in Greek and palavers with the dead, is a stunner."
On 14 May 2013 Ali Smith gave the inaugural Harriet Martineau lecture, in celebration of Norwich, UNESCO City of Literature.
Ali Smith is also a patron of the Visual Verse online anthology and her piece Untitled, written in response to an image by artist Rupert Jessop, appears in the November 2014 edition.