Moore was a three-time NFL Champion, with the Packers in 1961, 1962, and 1965. He was selected for the 1962 Pro Bowl & all-pro selection in 1963. Moore was selected as Green Bay's first-round selection in 1960 (No. 5 overall). He wore jersey number #25 for the Packers.
Moore was second-leading rusher on team in 1962 (377 yards) and 1963 (658 yards) behind Jim Taylor. He cored career-high seven rushing touchdowns in 1962 season. He gained 2,069 yards on the ground and scored 20 rushing touchdowns and had 71 receptions for 605 yards and seven touchdowns. He played in 78 regular-season games for the Packers.