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She married Major Sir John Alexander Arnott, 2nd Bt. (16 November 1853 – 26 July 1940), son of Sir John Arnott, 1st Bt. and Mary (née McKinlay), on 27 September 1881. Major Sir John Arnott was of the Arnott baronets. He gained the title of 2nd Baronet Arnott, of Woodlands, Shandon, Co. Cork [U.K., 1896] on 28 March 1898. He gained the rank of Major in the service of the 4th Battalion, Cheshire Regiment. He gained the rank of Honorary Lieutenant-Colonel in the service of the 4th Battalion, Cheshire Regiment. He held the office of Justice of the Peace (JP) for County Cork and of Deputy Lieutenant (DL) of County Cork.
- Lina Victoria Arnott (d. 25 October 1974)
- Margaret Christian Salome Arnott (d. 14 March 1952)
- Mary Christian Arnott (d. 26 May 1936)
- Captain John Arnott (b. 25 July 1885 - d. 30 March 1918)
- Sir Lauriston John Arnott, 3rd Bt. (b. 27 November 1890 - d. 2 July 1958)
- Sir Robert John Arnott, 4th Bt. (b. 19 August 1896 - d. 25 July 1966)
- Major Thomas John Arnott (b. 12 April 1899 - d. 16 July 1979)
She was invested as a Lady of Grace, Order of St John of Jerusalem (LGStJ). She held the office of Justice of the Peace (JP). She was invested as a Dame Commander of the Order of the British Empire)[why?] in 1918.
Dame Caroline Arnott died on 28 December 1933 of unknown causes.[where?]
- Charles Mosley, editor, Burke's Peerage, Baronetage & Knightage, 107th edition, 3 vol. (Wilmington, Delaware: Burke's Peerage (Genealogical Books) Ltd, 2003); vol. 1, p. 142.
- Profile, Peerage.com; accessed 20 March 2016.