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- Theophylact Simocatta, 7th century Byzantine author and historian
- Theophylactus (Exarch) (d. 710), Exarch of Ravenna
- Patriarch Theophylactus of Alexandria, coadjutor Greek Orthodox Patriarch of Alexandria (c. 695 - c. 711)
- Theophylact of Antioch, Orthodox Patriarch of Antioch (744-751)
- Theophylact (son of Michael I), Byzantine co-emperor 811–813
- Theophylact of Nicomedia, bishop of Nicomedia (d. 845 AD)
- Patriarch Theophylactus of Constantinople (917-956), Patriarch of Constantinople
- Pope Benedict VIII (d. 1024), born Theophylactus
- Pope Benedict IX (born c. 1012; d. between 1055 and 1056); born Theophylactus
- Theophylact of Ohrid (d. c. 1107), Archbishop of Ohrid and biblical commentator
- Peter of Atroa, who was born with the name Theophylact
- Theophylact, Count of Tusculum
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